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I'm not sure what you're trying to achieve. An NDR is a sign that something is wrong with email delivery, so things like filling the mailbox up would achieve the same result.
In theory, you could try spoofing an NDR using a carefully-worded auto-reply rule. However, this would appear as sent by the target mailbox, not by the System Administrator or Postmaster.
Do you have comments on this Ask the Expert Q&A? Let us know.
Related information from SearchExchange.com:
Tip: Customize non-delivery reports for MAPI messages
Tip: Dealing with undeliverable messages in Exchange Server
Tip: Troubleshooting non-delivery reports
Expert Advice: How to designate NDR recipients
15 tips in 15 minutes: Managing recipients and distribution lists
Reference Center: Non-delivery reports (NDRs) advice and resources
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